Artículo

Estamos trabajando para incorporar este artículo al repositorio
Consulte el artículo en la página del editor
Consulte la política de Acceso Abierto del editor

Abstract:

Highly ordered mesoporous ZrO2 thin films were prepared by evaporation induced self-assembly. Complexing agents and low pH were simultaneously employed in order to control the hydrolysis-condensation kinetics, permitting to cast films in one step. Many commercially available PPO-based surfactants can be used as templates, yielding different pore sizes. The mesoporosity is well preserved at high temperatures (600 °C) and after exposing the films to extreme alkaline conditions (1 M NaOH, 18 h). The procedure has been used to cast multilayer films, paving the way to mesoporous thin films-based UV photonics. © The Royal Society of Chemistry 2013.

Registro:

Documento: Artículo
Título:One-step preparation of UV transparent highly ordered mesoporous zirconia thin films
Autor:Zelcer, A.; Soler-Illia, G.J.A.A.
Filiación:Escuela de Ciencia y Tecnología, Universidad Nacional de San Martín, Argentina
Gerencia Química, Centro Atómico Constituyentes, Comisión Nacional de Energía Atómica, Av. Gral Paz 1499, B1650KNA, Argentina
DQIAyQF, FCEyN, Universidad de Buenos Aires, Argentina
Palabras clave:Alkalinity; Multilayer films; Thin films; Zirconia; Alkaline conditions; Cast film; Complexing agents; Different pore sizes; High temperature; Mesoporosity; Mesoporous; Ordered mesoporous; Mesoporous materials
Año:2013
Volumen:1
Número:7
Página de inicio:1359
Página de fin:1367
DOI: http://dx.doi.org/10.1039/c2tc00319h
Título revista:Journal of Materials Chemistry C
Título revista abreviado:J. Mater. Chem. C
ISSN:20507534
CODEN:JMCCC
Registro:https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_20507534_v1_n7_p1359_Zelcer

Referencias:

  • (2008) Chem. Mater., 20 (3)
  • Calvo, A., Yameen, B., Williams, F.J., Soler-Illia, G.J.A.A., Azzaroni, O., (2009) J. Am. Chem. Soc., 131, p. 10866
  • Otal, E.H., Angelomé, P.C., Bilmes, S.A., Soler-Illia, G.J.A.A., (2006) Adv. Mater., 18, p. 934
  • Choi, S.Y., Mamak, M., Von Freymann, G., Chopra, N., Ozin, G.A., (2006) Nano Lett., 6, p. 2456
  • Fuertes, M.C., López-Alcaraz, F.J., Marchi, M.C., Troiani, H.E., Luca, V., Míguez, H., Soler-Illia, G.J.A.A., (2007) Adv. Funct. Mater., 17, p. 1247
  • Sanchez, C., Boissiere, C., Grosso, D., Laberty, C., Nicole, L., (2008) Chem. Mater., 20, p. 682
  • Brinker, C.J., Lu, Y., Sellinger, A., Fan, H., (1999) Adv. Mater., 11, p. 579
  • Grosso, D., Cagnol, F., Soler-Illia, G.J.A.A., Crepaldi, E.L., Amenitsch, H., Brunet-Bruneau, A., Bourgeois, A., Sanchez, C., (2004) Adv. Funct. Mater., 14, p. 309
  • Soler-Illia, G.J.A.A., Innocenzi, P., (2006) Chem.-Eur. J., 12, p. 4478
  • Soler-Illia, G.J.A.A., Scolan, E., Louis, A., Albouy, P.-A., Sanchez, C., (2001) New J. Chem., 25, p. 156
  • Soler-Illia, G.J.A.A., Sanchez, C., (2000) New J. Chem., 24, p. 493
  • Soler-Illia, G.J.A.A., Angelomé, P.C., Fuertes, M.C., Grosso, D., Boissiere, C., (2012) Nanoscale, 4, p. 2549
  • Dunphy, D.R., Singer, S., Cook, A.W., Smarsly, B., Doshi, D.A., Brinker, C.J., (2003) Langmuir, 19, p. 10403
  • Bass, J.D., Grosso, D., Boissiere, C., Belamie, E., Coradin, T., Sanchez, C., (2007) Chem. Mater., 19, p. 4349
  • Liu, G., Lin, Y., (2005) Anal. Chem., 77, p. 5894
  • Queffélec, C., Petit, M., Janvier, P., Knight, D.A., Bujoli, B., (2012) Chem. Rev., 112, p. 3777
  • Izumi, K., Murakami, M., Deguchi, T., Morita, A., Tohge, N., Minami, T., (1989) J. Am. Ceram. Soc., 72, p. 1465
  • Crepaldi, E.L., Soler-Illia, G.J.A.A., Grosso, D., Sanchez, C., (2003) New J. Chem., 27, p. 9
  • Crepaldi, E.L., Soler-Illia, G.J.A.A., Bouchara, A., Grosso, D., Durand, D., Sanchez, C., (2003) Angew. Chem., Int. Ed., 42, p. 347
  • Brezesinski, T., Antonietti, M., Groenewolt, M., Pinna, N., Smarsly, B., (2005) New J. Chem., 29, p. 237
  • Fang, H., Wan, T., Shi, W., Zhang, M., (2007) J. Non-Cryst. Solids, 353, p. 1657
  • Wang, K., Morris, M.A., Holmes, J.D., Yu, J., Xu, R., (2009) Microporous Mesoporous Mater., 117, p. 161
  • Soo, M.T., Kawamura, G., Muto, H., Cheong, K.Y., Lockman, Z., Noor, A.F.M., Matsuda, A., (2011) J. Ceram. Soc. Jpn., 119, p. 517
  • Fan, J., Boettcher, S.W., Stucky, G.D., (2006) Chem. Mater., 18, p. 6391
  • Boettcher, S.W., Bartl, M.H., Hu, J.G., Stucky, G.D., (2005) J. Am. Chem. Soc., 127, p. 9721
  • Beitollahi, A., Daie, A.H.H., Samie, L., Akbarnejad, M.M., (2010) J. Alloys Compd., 490, p. 311
  • Zhang, J., Deng, Y., Gu, D., Wang, S., She, L., Che, R., Wang, Z.-S., Zhao, D., (2011) Adv. Energy Mater., 1, p. 241
  • Yun, H.-S., Miyazawa, K., Zhou, H., Honma, I., Kuwabara, M., (2001) Adv. Mater., 13, p. 1377
  • Mitra, A., Jana, D., De, G., (2012) Microporous Mesoporous Mater., 158, p. 187
  • Mitra, A., Jana, D., De, G., (2012) Chem. Commun., 48, p. 3333
  • Soler-Illia, G.J.A.A., Crepaldi, E.L., Grosso, D., Sanchez, C., (2003) Curr. Opin. Colloid Interface Sci., 8, p. 109
  • Kern, W., Puotinen, D.A., (1970) RCA Rev., 31, p. 187
  • Gibaud, A., Vignaud, G., (2009) X-ray and Neutron Reflectivity: Principles and Applications, p. 94. , ed. J. Daillant and A. Gibaud, Springer, Berlin Heidelberg, ch. 3
  • Boissiere, C., Grosso, D., Lepoutre, S., Nicole, L., Brunet-Bruneau, A., Sanchez, C., (2005) Langmuir, 21, p. 12362
  • Sanchez, C., Soler-Illia, G.J.A.A., Ribot, F., Grosso, D., (2003) C. R. Chim., 6, p. 1131
  • Soler-Illia, G.J.A.A., Sanchez, C., Lebeau, B., Patarin, J., (2002) Chem. Rev., 102, p. 4093
  • Jolivet, J.-P., (2000) Metal Oxide Chemistry and Synthesis, , John Wiley and Sons
  • Pierre, A.C., (1998) Introduction to Sol-Gel Processing, , Kluwer Academic Publishers
  • Sanchez, C., Livage, J., Henry, M., Babonneau, F., (1988) J. Non-Cryst. Solids, 100, pp. 65-76
  • Soler-Illia, G.J.A.A., Crepaldi, E.L., Grosso, D., Durand, D., Sanchez, C., (2002) Chem. Commun., p. 2298
  • Soler-Illia, G.J.A.A., Crepaldi, E.L., Grosso, D., Sanchez, C., (2004) J. Mater. Chem., 14, p. 1879
  • Chougnet, A., Heitz, C., Søndergard, E., Berquier, J.-M., Albouy, P.-A., Klotz, M., (2005) J. Mater. Chem., 15, p. 3340
  • Angelomé, P.C., (2008), Ph.D. thesis, University of Buenos Aires; Lowell, S., Shields, J.E., Thomas, M.A., Thommes, M., (2004) Characterization of Porous Solids and Powders: Surface Area, Pore Size and Density, , Springer, 1st edn
  • Brinker, C.J., Scherer, G.W., (1990) Sol-Gel Science: The Physics and Chemistry of Sol-Gel Processing, , Academic Press Inc, San Diego, 1st edn
  • Faustini, M., Louis, B., Albouy, P.-A., Kuemmel, M., Grosso, D., (2010) J. Phys. Chem. C, 114, p. 7637
  • Chatry, M., Henry, M., In, M., Sanchez, C., Livage, J., (1994) J. Sol-Gel Sci. Technol., 1, p. 233
  • Socrates, G., (2004) Infrared and Raman Characteristic Group Frequencies, , John Wiley and Sons, 3rd edn
  • Grosso, D., Soler-Illia, G.J.A.A., Crepaldi, E.L., Cagnol, F., Sinturel, C., Bourgeois, A., Brunet-Bruneau, A., Sanchez, C., (2003) Chem. Mater., 15, p. 4562
  • Sakatani, Y., Grosso, D., Nicole, L., Boissière, C., Soler-Illia, G.J.A.A., Sanchez, C., (2006) J. Mater. Chem., 16, p. 77
  • Huo, Q., Margolese, D.I., Ciesla, U., Demuth, D.G., Feng, P., Gier, T.E., Sieger, P., Chmelka, B.F., (1994) Chem. Mater., 6, p. 1176

Citas:

---------- APA ----------
Zelcer, A. & Soler-Illia, G.J.A.A. (2013) . One-step preparation of UV transparent highly ordered mesoporous zirconia thin films. Journal of Materials Chemistry C, 1(7), 1359-1367.
http://dx.doi.org/10.1039/c2tc00319h
---------- CHICAGO ----------
Zelcer, A., Soler-Illia, G.J.A.A. "One-step preparation of UV transparent highly ordered mesoporous zirconia thin films" . Journal of Materials Chemistry C 1, no. 7 (2013) : 1359-1367.
http://dx.doi.org/10.1039/c2tc00319h
---------- MLA ----------
Zelcer, A., Soler-Illia, G.J.A.A. "One-step preparation of UV transparent highly ordered mesoporous zirconia thin films" . Journal of Materials Chemistry C, vol. 1, no. 7, 2013, pp. 1359-1367.
http://dx.doi.org/10.1039/c2tc00319h
---------- VANCOUVER ----------
Zelcer, A., Soler-Illia, G.J.A.A. One-step preparation of UV transparent highly ordered mesoporous zirconia thin films. J. Mater. Chem. C. 2013;1(7):1359-1367.
http://dx.doi.org/10.1039/c2tc00319h