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Caldarola, M.; Albella, P.; Cortés, E.; Rahmani, M.; Roschuk, T.; Grinblat, G.; Oulton, R.F.; Bragas, A.V.; Maier, S.A. "Non-plasmonic nanoantennas for surface enhanced spectroscopies with ultra-low heat conversion" (2015) Nature Communications. 6
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Abstract:

Nanoplasmonics has recently revolutionized our ability to control light on the nanoscale. Using metallic nanostructures with tailored shapes, it is possible to efficiently focus light into nanoscale field 'hot spots'. High field enhancement factors have been achieved in such optical nanoantennas, enabling transformative science in the areas of single molecule interactions, highly enhanced nonlinearities and nanoscale waveguiding. Unfortunately, these large enhancements come at the price of high optical losses due to absorption in the metal, severely limiting real-world applications. Via the realization of a novel nanophotonic platform based on dielectric nanostructures to form efficient nanoantennas with ultra-low light-into-heat conversion, here we demonstrate an approach that overcomes these limitations. We show that dimer-like silicon-based single nanoantennas produce both high surface enhanced fluorescence and surface enhanced Raman scattering, while at the same time generating a negligible temperature increase in their hot spots and surrounding environments. © 2015 Macmillan Publishers Limited. All rights reserved.

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Documento: Artículo
Título:Non-plasmonic nanoantennas for surface enhanced spectroscopies with ultra-low heat conversion
Autor:Caldarola, M.; Albella, P.; Cortés, E.; Rahmani, M.; Roschuk, T.; Grinblat, G.; Oulton, R.F.; Bragas, A.V.; Maier, S.A.
Filiación:Laboratorio de Electrónica Cuántica, Departamento de Física, FCEN, Universidad de Buenos Aires, Intendente Güiraldes 2160, Buenos Aires, Argentina - IFIBA CONICET, C1428EGA, Argentina
Blackett Laboratory, Department of Physics, Imperial College London, London, SW7 2AZ, United Kingdom
Palabras clave:dimer; gold; nanomaterial; silicon; fluorescence; heat balance; light effect; molecular analysis; nonlinearity; optical property; Raman spectroscopy; silicon; spectroscopy; temperature effect; Article; electromagnetic field; fluorescence; heating; molecular electronics; nanofabrication; Raman spectrometry; spectroscopy; temperature
Año:2015
Volumen:6
DOI: http://dx.doi.org/10.1038/ncomms8915
Título revista:Nature Communications
Título revista abreviado:Nat. Commun.
ISSN:20411723
CAS:gold, 7440-57-5; silicon, 7440-21-3
Registro:https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_20411723_v6_n_p_Caldarola

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Citas:

---------- APA ----------
Caldarola, M., Albella, P., Cortés, E., Rahmani, M., Roschuk, T., Grinblat, G., Oulton, R.F.,..., Maier, S.A. (2015) . Non-plasmonic nanoantennas for surface enhanced spectroscopies with ultra-low heat conversion. Nature Communications, 6.
http://dx.doi.org/10.1038/ncomms8915
---------- CHICAGO ----------
Caldarola, M., Albella, P., Cortés, E., Rahmani, M., Roschuk, T., Grinblat, G., et al. "Non-plasmonic nanoantennas for surface enhanced spectroscopies with ultra-low heat conversion" . Nature Communications 6 (2015).
http://dx.doi.org/10.1038/ncomms8915
---------- MLA ----------
Caldarola, M., Albella, P., Cortés, E., Rahmani, M., Roschuk, T., Grinblat, G., et al. "Non-plasmonic nanoantennas for surface enhanced spectroscopies with ultra-low heat conversion" . Nature Communications, vol. 6, 2015.
http://dx.doi.org/10.1038/ncomms8915
---------- VANCOUVER ----------
Caldarola, M., Albella, P., Cortés, E., Rahmani, M., Roschuk, T., Grinblat, G., et al. Non-plasmonic nanoantennas for surface enhanced spectroscopies with ultra-low heat conversion. Nat. Commun. 2015;6.
http://dx.doi.org/10.1038/ncomms8915