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Morozov, Y.V.; Draguta, S.; Zhang, S.; Cadranel, A.; Wang, Y.; Janko, B.; Kuno, M. "Defect-Mediated CdS Nanobelt Photoluminescence Up-Conversion" (2017) Journal of Physical Chemistry C. 121(30):16607-16616
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Abstract:

Laser cooling in semiconductors has recently been demonstrated in cadmium sulfide nanobelts (NBs) as well as in organic-inorganic lead halide perovskites. Cooling by as much as 40 K has been shown in CdS nanobelts and by as much as 58 K in hybrid perovskite films. This suggests that further progress in semiconductor-based optical refrigeration can ultimately lead to solid state cryocoolers capable of achieving sub 10 K temperatures. In CdS, highly efficient photoluminescence (PL) up-conversion has been attributed to efficient exciton-longitudinal optical (LO) phonon coupling. However, the nature of its efficient anti-Stokes emission has not been established. Consequently, developing a detailed understanding about the mechanism leading to efficient PL up-conversion in CdS NBs is essential to furthering the nascent field of semiconductor laser cooling. In this study, we describe a detailed investigation of anti-Stokes photoluminescence (ASPL) in CdS nanobelts. Temperature- and frequency-dependent band edge emission and ASPL spectroscopies conducted on individual belts as well as ensembles suggest that CdS ASPL is defect-mediated via the involvement of donor-acceptor states. © 2017 American Chemical Society.

Registro:

Documento: Artículo
Título:Defect-Mediated CdS Nanobelt Photoluminescence Up-Conversion
Autor:Morozov, Y.V.; Draguta, S.; Zhang, S.; Cadranel, A.; Wang, Y.; Janko, B.; Kuno, M.
Filiación:Department of Chemistry and Biochemistry, University of Notre Dame, 251 Nieuwland Science Hall, Notre Dame, IN 46556, United States
Department of Physics, University of Notre Dame, 225 Nieuwland Science Hall, Notre Dame, IN 46556, United States
Departamento de Química Analítica, Inorgánica y Química Física, INQUIMAE, Facultad de Ciencias Exactas y Naturales, Universidad de Buenos Aires, Pabellón 2, Ciudad Universitaria, Buenos Aires, C1428EHA, Argentina
Palabras clave:Cadmium sulfide; Cooling; Defects; Laser cooling; Nanobelts; Organic lasers; Perovskite; Photoluminescence; Semiconductor lasers; Semiconductor quantum wells; Anti-Stokes emission; Anti-Stokes photoluminescence; Band-edge emissions; Frequency dependent; Halide perovskites; Longitudinal optical phonons; Optical refrigeration; Organic-inorganic; II-VI semiconductors
Año:2017
Volumen:121
Número:30
Página de inicio:16607
Página de fin:16616
DOI: http://dx.doi.org/10.1021/acs.jpcc.7b05095
Título revista:Journal of Physical Chemistry C
Título revista abreviado:J. Phys. Chem. C
ISSN:19327447
Registro:https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_19327447_v121_n30_p16607_Morozov

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Citas:

---------- APA ----------
Morozov, Y.V., Draguta, S., Zhang, S., Cadranel, A., Wang, Y., Janko, B. & Kuno, M. (2017) . Defect-Mediated CdS Nanobelt Photoluminescence Up-Conversion. Journal of Physical Chemistry C, 121(30), 16607-16616.
http://dx.doi.org/10.1021/acs.jpcc.7b05095
---------- CHICAGO ----------
Morozov, Y.V., Draguta, S., Zhang, S., Cadranel, A., Wang, Y., Janko, B., et al. "Defect-Mediated CdS Nanobelt Photoluminescence Up-Conversion" . Journal of Physical Chemistry C 121, no. 30 (2017) : 16607-16616.
http://dx.doi.org/10.1021/acs.jpcc.7b05095
---------- MLA ----------
Morozov, Y.V., Draguta, S., Zhang, S., Cadranel, A., Wang, Y., Janko, B., et al. "Defect-Mediated CdS Nanobelt Photoluminescence Up-Conversion" . Journal of Physical Chemistry C, vol. 121, no. 30, 2017, pp. 16607-16616.
http://dx.doi.org/10.1021/acs.jpcc.7b05095
---------- VANCOUVER ----------
Morozov, Y.V., Draguta, S., Zhang, S., Cadranel, A., Wang, Y., Janko, B., et al. Defect-Mediated CdS Nanobelt Photoluminescence Up-Conversion. J. Phys. Chem. C. 2017;121(30):16607-16616.
http://dx.doi.org/10.1021/acs.jpcc.7b05095