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Abstract:

Large-size mesoporous thin films with a mixed titania-silica framework and an Im over(3, -) m cubic-derived or worm-like mesostructure were obtained by combining sol-gel and macromolecular templating techniques. These materials presented accessible mesopores (20 to 25% pore volume), tunable refractive index and high molecular-scale mixing of both ions, as demonstrated by UV-Visible, FTIR and XANES spectroscopy. In addition, a composition effect in the catalytic reduction of silver was found, which permitted one to obtain homogeneous metal nanoparticle-mesoporous film nanocomposites with tuned plasmon position. © 2009 Académie des sciences.

Registro:

Documento: Artículo
Título:Large-pore mesoporous titania-silica thin films (Ti1-xSixO2, 0.1 ≤ x ≤ 0.9) with highly interdispersed mixed oxide frameworks
Autor:Angelomé, P.C.; Andrini, L.; Fuertes, M.C.; Requejo, F.G.; Soler-Illia, G.J.A.A.
Filiación:Gerencia de Química, CNEA, Centro Atómico Constituyentes, Avenue Gral Paz 1499, San Martín, B1650KNA, Argentina
Departamento Física, FCE, UNLP and INIFTA-IFLP (CONICET), CC/67, 1900 La Plata, Argentina
CONICET, Avenue Rivadavia 1917, C1033AAJ Buenos Aires, Argentina
DQIAyQF, FCEN, Universidad de Buenos Aires, Ciudad Universitaria, Pabellon II, C1428EHA Buenos Aires, Argentina
Palabras clave:Catalysis; Mesoporous films; Mixed oxides; Self-assembly; Sol-gel
Año:2010
Volumen:13
Número:1-2
Página de inicio:256
Página de fin:269
DOI: http://dx.doi.org/10.1016/j.crci.2009.07.001
Título revista:Comptes Rendus Chimie
Título revista abreviado:C. R. Chim.
ISSN:16310748
CODEN:CRCOC
Registro:https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_16310748_v13_n1-2_p256_Angelome

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Citas:

---------- APA ----------
Angelomé, P.C., Andrini, L., Fuertes, M.C., Requejo, F.G. & Soler-Illia, G.J.A.A. (2010) . Large-pore mesoporous titania-silica thin films (Ti1-xSixO2, 0.1 ≤ x ≤ 0.9) with highly interdispersed mixed oxide frameworks. Comptes Rendus Chimie, 13(1-2), 256-269.
http://dx.doi.org/10.1016/j.crci.2009.07.001
---------- CHICAGO ----------
Angelomé, P.C., Andrini, L., Fuertes, M.C., Requejo, F.G., Soler-Illia, G.J.A.A. "Large-pore mesoporous titania-silica thin films (Ti1-xSixO2, 0.1 ≤ x ≤ 0.9) with highly interdispersed mixed oxide frameworks" . Comptes Rendus Chimie 13, no. 1-2 (2010) : 256-269.
http://dx.doi.org/10.1016/j.crci.2009.07.001
---------- MLA ----------
Angelomé, P.C., Andrini, L., Fuertes, M.C., Requejo, F.G., Soler-Illia, G.J.A.A. "Large-pore mesoporous titania-silica thin films (Ti1-xSixO2, 0.1 ≤ x ≤ 0.9) with highly interdispersed mixed oxide frameworks" . Comptes Rendus Chimie, vol. 13, no. 1-2, 2010, pp. 256-269.
http://dx.doi.org/10.1016/j.crci.2009.07.001
---------- VANCOUVER ----------
Angelomé, P.C., Andrini, L., Fuertes, M.C., Requejo, F.G., Soler-Illia, G.J.A.A. Large-pore mesoporous titania-silica thin films (Ti1-xSixO2, 0.1 ≤ x ≤ 0.9) with highly interdispersed mixed oxide frameworks. C. R. Chim. 2010;13(1-2):256-269.
http://dx.doi.org/10.1016/j.crci.2009.07.001