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Abstract:

This manuscript addresses the synthesis, structural characterization and optical properties of a 1D coordination polymer (CPs) and 2D and 3D Metal-Organic Frameworks (MOFs) obtained from lanthanide metals, 3-hydroxinaftalene-2,7-disulfonic acid (3-OHNDS) and two different phenanthroline derivates as ancillary ligands. The first is a family of 2D compounds with formula [Ln(3-OHNDS)(H2O)2], where Ln = La(1), Pr(2), Nd(3) and Sm(4). The addition of 1,10-phenanthroline (phen) in the reaction produces 1D compounds with general formula [Ln(3-OHNDS)(phen)(H2O)]·3H2O, where Ln = La(5), Pr(6), Nd(7) and Sm(8). Finally, the synthesis with 3,4,7,8-tetramethyl-1,10-phenanthroline (3,4,7,8-TMPhen) as an ancillary ligand results in the formation of the 3D [La(3-OHNDS)(3,4,7,8-TMphen)(H2O)] (9) compound. The photoluminescence (PL) properties of 1D and 2D compounds were fully investigated in comparison with the 3-OHNDS ligand. One of the most important results was the obtaining of a white-light single-emitter without adding dopant atoms in the structure. With all these results in mind it was possible to establish structure-property relationships. © 2016 The Royal Society of Chemistry.

Registro:

Documento: Artículo
Título:Tuning the structure, dimensionality and luminescent properties of lanthanide metal-organic frameworks under ancillary ligand influence
Autor:D'Vries, R.F.; Gomez, G.E.; Hodak, J.H.; Soler-Illia, G.J.A.A.; Ellena, J.
Filiación:Instituto de Física de São Carlos, Universidade de São Paulo, São Carlos SP, CEP. 13566-590, Brazil
Gerencia de Investigación y Aplicaciones, Centro Atómico Constituyentes, Comisión Nacional de Energía Atómica, Grupo de Nanoquímica, Av. Gral. Paz 1499, San Martin, Buenos Aires, 1650, Argentina
DQIAyQF, INQUIMAE-CONICET FCEN Universidad de Buenos Aires, Pab. II Ciudad Universitaria CABA1428, Buenos Aires, Argentina
Palabras clave:Chelation; Crystalline materials; Ligands; Optical properties; Organometallics; Rare earth elements; Structural metals; 1 ,10-phenanthroline; 1D coordination polymer; Ancillary ligands; Luminescent property; Metal organic framework; Photoluminescence properties; Structural characterization; Structure property relationships; Structural properties
Año:2016
Volumen:45
Número:2
Página de inicio:646
Página de fin:656
DOI: http://dx.doi.org/10.1039/c5dt04033g
Título revista:Dalton Transactions
Título revista abreviado:Dalton Trans.
ISSN:14779226
CODEN:DTARA
Registro:https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_14779226_v45_n2_p646_DVries

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Citas:

---------- APA ----------
D'Vries, R.F., Gomez, G.E., Hodak, J.H., Soler-Illia, G.J.A.A. & Ellena, J. (2016) . Tuning the structure, dimensionality and luminescent properties of lanthanide metal-organic frameworks under ancillary ligand influence. Dalton Transactions, 45(2), 646-656.
http://dx.doi.org/10.1039/c5dt04033g
---------- CHICAGO ----------
D'Vries, R.F., Gomez, G.E., Hodak, J.H., Soler-Illia, G.J.A.A., Ellena, J. "Tuning the structure, dimensionality and luminescent properties of lanthanide metal-organic frameworks under ancillary ligand influence" . Dalton Transactions 45, no. 2 (2016) : 646-656.
http://dx.doi.org/10.1039/c5dt04033g
---------- MLA ----------
D'Vries, R.F., Gomez, G.E., Hodak, J.H., Soler-Illia, G.J.A.A., Ellena, J. "Tuning the structure, dimensionality and luminescent properties of lanthanide metal-organic frameworks under ancillary ligand influence" . Dalton Transactions, vol. 45, no. 2, 2016, pp. 646-656.
http://dx.doi.org/10.1039/c5dt04033g
---------- VANCOUVER ----------
D'Vries, R.F., Gomez, G.E., Hodak, J.H., Soler-Illia, G.J.A.A., Ellena, J. Tuning the structure, dimensionality and luminescent properties of lanthanide metal-organic frameworks under ancillary ligand influence. Dalton Trans. 2016;45(2):646-656.
http://dx.doi.org/10.1039/c5dt04033g