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Krause, S.; Aramendia, P.F.; Täuber, D.; Von Borczyskowski, C. "Freezing single molecule dynamics on interfaces and in polymers" (2011) Physical Chemistry Chemical Physics. 13(5):1754-1761
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Abstract:

Heterogeneous line broadening and spectral diffusion of the fluorescence emission spectra of perylene diimide molecules have been investigated by means of time dependent single molecule spectroscopy. The influence of temperature and environment has been studied and reveals strong correlation to spectral diffusion processes. We followed the freezing of the molecular mobility of quasi free molecules on the surface upon temperature lowering and by embedding into a poly(methyl methacrylate) (PMMA) polymer. Thereby changes of optical transition energies as a result of both intramolecular changes of conformation and external induced dynamics by the surrounding polymer matrix could be observed. Simulations of spectral fluctuations within a two-level system (TLS) model showed good agreement with the experimental findings. © the Owner Societies.

Registro:

Documento: Artículo
Título:Freezing single molecule dynamics on interfaces and in polymers
Autor:Krause, S.; Aramendia, P.F.; Täuber, D.; Von Borczyskowski, C.
Filiación:Institute of Physics and NanoMA, Center for Nanostructured Materials and Analysis, Chemnitz University of Technology, 09107 Chemnitz, Germany
Dept. Química Inorgánica, Universidad de Buenos Aires, C1428EHA Buenos Aires, Argentina
Año:2011
Volumen:13
Número:5
Página de inicio:1754
Página de fin:1761
DOI: http://dx.doi.org/10.1039/c0cp01713b
Título revista:Physical Chemistry Chemical Physics
Título revista abreviado:Phys. Chem. Chem. Phys.
ISSN:14639076
CODEN:PPCPF
Registro:https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_14639076_v13_n5_p1754_Krause

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Citas:

---------- APA ----------
Krause, S., Aramendia, P.F., Täuber, D. & Von Borczyskowski, C. (2011) . Freezing single molecule dynamics on interfaces and in polymers. Physical Chemistry Chemical Physics, 13(5), 1754-1761.
http://dx.doi.org/10.1039/c0cp01713b
---------- CHICAGO ----------
Krause, S., Aramendia, P.F., Täuber, D., Von Borczyskowski, C. "Freezing single molecule dynamics on interfaces and in polymers" . Physical Chemistry Chemical Physics 13, no. 5 (2011) : 1754-1761.
http://dx.doi.org/10.1039/c0cp01713b
---------- MLA ----------
Krause, S., Aramendia, P.F., Täuber, D., Von Borczyskowski, C. "Freezing single molecule dynamics on interfaces and in polymers" . Physical Chemistry Chemical Physics, vol. 13, no. 5, 2011, pp. 1754-1761.
http://dx.doi.org/10.1039/c0cp01713b
---------- VANCOUVER ----------
Krause, S., Aramendia, P.F., Täuber, D., Von Borczyskowski, C. Freezing single molecule dynamics on interfaces and in polymers. Phys. Chem. Chem. Phys. 2011;13(5):1754-1761.
http://dx.doi.org/10.1039/c0cp01713b