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Abstract:

The coordination of PySSPy to FePc was monitored by UV/Vis spectroscopy while the adsobed FePc, anchored by PyS−Au(111), was examined by in situ STM in 0.1 M HClO4 and X-ray photoelectron spectroscopy (XPS). Rotating-disc-electrode (RDE) and linear-sweep-voltammetry (LSV) studies on the resulting FePc-modified Au(111) electrodes in an oxygen-saturated 0.1 M NaOH electrolyte exhibit excellent electrocatalytic properties for the oxygen reduction reaction (ORR), with a smaller overpotential than that observed for Au(111) with FePc deposited by direct adsorption from a benzene solution. © 2018 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim

Registro:

Documento: Artículo
Título:Adsorption of 4,4′-Dithiodipyridine Axially Coordinated to Iron(II) Phthalocyanine on Au(111) as a New Strategy for Oxygen Reduction Electrocatalysis
Autor:Herrera, S.; Tasca, F.; Williams, F.J.; Calvo, E.J.
Filiación:Department of Inorganic Chemistry, Analytical and Chemical Physics, INQUIMAE-CONICET, Facultad de Ciencias Exactas y Naturales, Universidad de Buenos Aires Ciudad Universitaria, Pabellón 2, Buenos Aires, C1428EHA, Argentina
Department of Chemistry Materials, Facultad de Química y Biología, Universidad de Santiago de Chile, Av. Libertador Bernardo O'Higgins, Santiago, 3363, Chile
Palabras clave:electrocatalysis; oxygen reduction reaction; phthalocyanines; scanning tunnelling microscopy; X-ray spectroscopy
Año:2018
Volumen:19
Número:13
Página de inicio:1599
Página de fin:1604
DOI: http://dx.doi.org/10.1002/cphc.201800139
Título revista:ChemPhysChem
Título revista abreviado:ChemPhysChem
ISSN:14394235
CODEN:CPCHF
Registro:https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_14394235_v19_n13_p1599_Herrera

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Citas:

---------- APA ----------
Herrera, S., Tasca, F., Williams, F.J. & Calvo, E.J. (2018) . Adsorption of 4,4′-Dithiodipyridine Axially Coordinated to Iron(II) Phthalocyanine on Au(111) as a New Strategy for Oxygen Reduction Electrocatalysis. ChemPhysChem, 19(13), 1599-1604.
http://dx.doi.org/10.1002/cphc.201800139
---------- CHICAGO ----------
Herrera, S., Tasca, F., Williams, F.J., Calvo, E.J. "Adsorption of 4,4′-Dithiodipyridine Axially Coordinated to Iron(II) Phthalocyanine on Au(111) as a New Strategy for Oxygen Reduction Electrocatalysis" . ChemPhysChem 19, no. 13 (2018) : 1599-1604.
http://dx.doi.org/10.1002/cphc.201800139
---------- MLA ----------
Herrera, S., Tasca, F., Williams, F.J., Calvo, E.J. "Adsorption of 4,4′-Dithiodipyridine Axially Coordinated to Iron(II) Phthalocyanine on Au(111) as a New Strategy for Oxygen Reduction Electrocatalysis" . ChemPhysChem, vol. 19, no. 13, 2018, pp. 1599-1604.
http://dx.doi.org/10.1002/cphc.201800139
---------- VANCOUVER ----------
Herrera, S., Tasca, F., Williams, F.J., Calvo, E.J. Adsorption of 4,4′-Dithiodipyridine Axially Coordinated to Iron(II) Phthalocyanine on Au(111) as a New Strategy for Oxygen Reduction Electrocatalysis. ChemPhysChem. 2018;19(13):1599-1604.
http://dx.doi.org/10.1002/cphc.201800139