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De Tendler, R.H.; Barbiric, D.A.; Rodriguez, C.; Kovacs, J.A.; Pepe, M.E.; Gallego, L.J.; Alonso, J.A. "Theoretical analysis of the glass-forming behaviour of Ni-Zr and Ni-Zr-Fe alloys" (2000) International Journal of Non-Equilibrium Processing. 11(3):299-322
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Abstract:

The metastable free energy diagram of the Ni-Zr alloy at 300 K was calculated using Miedema's theory. A previous extension of the theory to ternary systems was further developed and used to calculate the free energies of the metastable amorphous phase and crystalline solid solutions of the Ni-Zr-Fe system at 300 K. The results of the calculations are compared with experimental data taken from the literature. The metastable free energy diagram of Ni-Zr is consistent with the measured glass-forming range. It allows to predict the succession of phases - amorphous alloys, crystalline solid solutions and intermetallic compounds - observed in rapidly quenched Ni-Zr alloys and in solid-state interdiffusion in Ni-Zr composites. In the ternary system Ni-Zr-Fe, intersections of the calculated free-energy surfaces of solid solutions together with that of the amorphous phase define an extended glass-forming composition range that contains the observed Ni-Zr-Fe glass compositions. The relative positions of the free-energy surfaces of the bcc solid solution and the amorphous phase and the region of metastable equilibrium between amorphous alloy and α-Zr solid solution provide the basis for interpreting the appearance of different phases in experiments on partial amorphization of Zr-rich, Ni-Zr-Fe melt-quenched alloys.

Registro:

Documento: Artículo
Título:Theoretical analysis of the glass-forming behaviour of Ni-Zr and Ni-Zr-Fe alloys
Autor:De Tendler, R.H.; Barbiric, D.A.; Rodriguez, C.; Kovacs, J.A.; Pepe, M.E.; Gallego, L.J.; Alonso, J.A.
Ciudad:Oxon, United Kingdom
Filiación:Inst. Univ. de Estudios Nucleares, Centro Atómico Ezeiza, Coḿn. Nac. de Ener. Atomica, Avenida del Libertador 8250, 1429 Buenos Aires, Argentina
Depto. Quim. Inorg., Analitica Q., Fac. de Ciencias Exactas y Naturales, Ciudad Universitaria, 1428 Buenos Aires, Argentina
Secretaria de Cie. y Tecnica, Facultad Regional Buenos Aires, Univ. Tecnólogica Nacional, Medrano 951, 1179 Buenos Aires, Argentina
General Industries Argentina S.A., Ituzaingó 270, Córdoba, Argentina
Serv. de Info. y Comunicaciones, Centro Atómico Constituyentes, Coḿn. Nac. de Ener. Atomica, Avenida del Libertador 8250, 1429 Buenos Aires, Argentina
Depto. Fis. Materia Condensada, Facultad de Física, Univ. de Santiago de Compostela, Santiago de Compostela, La Coruna, Spain
Depto. de Fisica Teórica, Facultad de Ciencias, Universidad de Valladolid, Valladolid 47011, Spain
Palabras clave:Gibbs free energy; Glass transition; Intermetallics; Mathematical models; Nickel alloys; Solid solutions; Temperature; Complete glass forming range; Extended glass forming range; Glass forming behavior; Miedema theory; Amorphous alloys
Año:2000
Volumen:11
Número:3
Página de inicio:299
Página de fin:322
Título revista:International Journal of Non-Equilibrium Processing
Título revista abreviado:Int J Non Equilibrium Process
ISSN:13689290
CODEN:IJNPF
Registro:https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_13689290_v11_n3_p299_DeTendler

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Citas:

---------- APA ----------
De Tendler, R.H., Barbiric, D.A., Rodriguez, C., Kovacs, J.A., Pepe, M.E., Gallego, L.J. & Alonso, J.A. (2000) . Theoretical analysis of the glass-forming behaviour of Ni-Zr and Ni-Zr-Fe alloys. International Journal of Non-Equilibrium Processing, 11(3), 299-322.
Recuperado de https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_13689290_v11_n3_p299_DeTendler [ ]
---------- CHICAGO ----------
De Tendler, R.H., Barbiric, D.A., Rodriguez, C., Kovacs, J.A., Pepe, M.E., Gallego, L.J., et al. "Theoretical analysis of the glass-forming behaviour of Ni-Zr and Ni-Zr-Fe alloys" . International Journal of Non-Equilibrium Processing 11, no. 3 (2000) : 299-322.
Recuperado de https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_13689290_v11_n3_p299_DeTendler [ ]
---------- MLA ----------
De Tendler, R.H., Barbiric, D.A., Rodriguez, C., Kovacs, J.A., Pepe, M.E., Gallego, L.J., et al. "Theoretical analysis of the glass-forming behaviour of Ni-Zr and Ni-Zr-Fe alloys" . International Journal of Non-Equilibrium Processing, vol. 11, no. 3, 2000, pp. 299-322.
Recuperado de https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_13689290_v11_n3_p299_DeTendler [ ]
---------- VANCOUVER ----------
De Tendler, R.H., Barbiric, D.A., Rodriguez, C., Kovacs, J.A., Pepe, M.E., Gallego, L.J., et al. Theoretical analysis of the glass-forming behaviour of Ni-Zr and Ni-Zr-Fe alloys. Int J Non Equilibrium Process. 2000;11(3):299-322.
Available from: https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_13689290_v11_n3_p299_DeTendler [ ]