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Abstract:

The electric susceptibility of neutral sodium-doped water clusters Na(H2ON, N = 6-33, was determined by beam electric deflection. The clusters behave as polarizable particles; their intensity profiles exhibit global shifts toward the high-field region without the occurrence of broadening. In the conditions of the experiment, sodium-water clusters have a "floppy" structure and hence the electric susceptibility presents both electronic and orientacional terms. Measured susceptibilities are somewhat higher than those of pure water clusters, and the contribution per water molecule is similar for both cluster types. © 2009 American Chemical Society.

Registro:

Documento: Artículo
Título:Electric susceptibility of sodium-doped water clusters by beam deflection
Autor:Carrera, Á.; Mobbili, M.; Marceca, E.
Filiación:INQUIMAE-DQIAQF, Facultad de Ciencias Exactas y Naturales, Ciudad Universitaria, Pabellón II, Buenos Aires, Argentina
Palabras clave:Beam deflections; Electric deflections; Electric susceptibilities; Global shifts; High-field regions; Intensity profiles; Polarizable particles; Pure waters; Water clusters; Water molecules; Sodium
Año:2009
Volumen:113
Número:12
Página de inicio:2711
Página de fin:2714
DOI: http://dx.doi.org/10.1021/jp809411p
Título revista:Journal of Physical Chemistry A
Título revista abreviado:J Phys Chem A
ISSN:10895639
CODEN:JPCAF
Registro:https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_10895639_v113_n12_p2711_Carrera

Referencias:

  • Broyer, M., Antoine, R., Benichou, E., Compagnon, I., Dugourd, P., (2002) C. R. Phys, 3, p. 301. , and references cited therein
  • Broyer, M., Antoine, R., Compagnon, I., Rayane, D., Dugourd, P., (2007) hys. Scr, 76. , C135, and references cited therein
  • Compagnon, I., Antoine, R., Rayane, D., Broyer, M., Dugourd, P., (2002) Phys. Rev. Lett, 89, p. 253001
  • Antoine, R., Compagnon, I., Rayane, D., Broyer, M., Dugourd, P., Breaux, G., Hagemeister, F.C., Jarrold, M.F., (2002) Eur. Phys. J. D, 20, p. 583
  • Moro, R., Rabinovitch, R., Xia, C., Kresin, V.V., (2006) Phys. Rev. Lett, 97, p. 123401
  • Hertel, I.V., Hiiglin, C., Nitsch, C., Schulz, C.P., (1991) Phys. Rev. Lett, 67, p. 1767
  • Schulz, C.P., Bobbert, C., Shimosato, T., Daigoku, K., Miura, N., Hashimoto, K., (2003) J. Chem. Phys, 119, p. 11620
  • Steinbach, C., Buck, U., (2006) J. Phys. Chem. A, 110, p. 3128
  • Barnett, R.N., Landman, U., (1993) Phys. Rev. Lett, 70, p. 1775
  • Tsurusawa, T., Iwata, S., (1999) J. Phys. Chem. A, 103, p. 6134
  • Ferro, Y., Allouche, A., (2003) J. Chem. Phys, 118, p. 10461
  • Gao, B., Liu, Z.F., (2007) J. Chem. Phys, 126, p. 084501
  • Buck, U., Dauster, I., Gao, B., Liu, Z.-F., (2007) J. Phys. Chem. A, 111, p. 12355
  • Bobbert, C., Schulz, C.P., (2001) Eur. Phys. J. D, 16, p. 95
  • Steinbach, C., Buck, U., (2005) J. Chem. Phys, 122, p. 134301
  • Bewig, L., Buck, U., Rakowswsky, S., Reymann, M., Steinbach, C., (1998) J. Phys. Chem. A, 102, p. 1124
  • Ramsey, N.F., (1956) Molecular beams, , Clarendon Press: Oxford, UK, and references therein
  • Aroney, M.J., Pattern, S.J., (1984) J. Chem. Soc, Faraday Trans, 80, p. 1201
  • Schäfer, S., Heiles, S., Becker, J.A., Schafer, R., (2008) J. Chem. Phys, 129, p. 044304
  • Rost, J.M., Griffin, J.C., Friedrich, B., Herschbach, D.R., (1992) Phys. Rev. Lett, 68, p. 1299
  • Benichou, E., Allouche, A.R., Antoine, R., Aubert-Frecon, M., Bourgoin, M., Broyer, M., Dugourd, P., Rayane, D., (2000) Eur. Phys. J. D, 10, p. 233
  • Dugourd, P., Compagnon, I., Lepine, F., Antoine, R., Rayane, D., Broyer, M., (2001) Chem. Phys. Lett, 336, p. 511
  • Bulthuis, J., Becker, J.A., Moro, R., Kresin, V.V., (2008) J. Chem. Phys, 129, p. 024101
  • Abd El Rahim, M., Antoine, R., Broyer, M., Rayane, D., Dugourd, P., (2005) J. Phys. Chem. A, 109, p. 8507
  • Dugourd, P., Antoine, R., Abd El Rahim, M., Rayane, D., Broyer, M., Calvo, F., (2006) Chem. Phys. Lett, 423, p. 13
  • Compagnon, I., Antoine, R., Rayane, D., Broyer, M., Dugourd, P., (2003) J. Phys. Chem. A, 107, p. 3036
  • Carrena, A., Mobbili, M., Moriena, G., Marceca, E., (2008) Chem. Phys. Lett, 467, p. 14
  • Schäfer, S., Schäfer, R., (2008) Phys. Rev. B, 77, p. 205211
  • Kittel, C., (1967) Introduction to Solid State Physics, , 3rd ed, Wiley: New York
  • Farley, F.W., McClelland, G.M., (1990) Science, 247, p. 1572
  • Rayane, D., Antoine, R., Dugourd, P., Benichou, E., Allouche, A.R., Aubert-Frécon, M., Broyer, M., (2000) Phys. Rev. Lett, 84, p. 1962
  • Frisch, M. J, Trucks, G. W, Schlegel, H. B, Scuseria, G. E, Robb, M. A, Cheeseman, J. R, Zakrzewski, V. G, Montgomery, J. A, Jr, Stratmann, R. E, Burant, J. C; Dapprich, S, Millam, J. M, Daniels, A. D, Kudin, K. N, Strain, M. C; Farkas, O, Tomasi, J, Barone, V, Cossi, M, Cammi, R, Mennucci, B, Pomelli, C; Adamo, C; Clifford, S, Ochterski, J, Petersson, G. A, Ayala, P. Y, Cui, Q, Morokuma, K, Malick, D. K, Rabuck, A. D, Raghavachari, K, Foresman, J. B, Cioslowski, J, Ortiz, J. V, Stefanov, B. B, Liu, G, Liashenko, A, Piskorz, P, Komaromi, I, Gomperts, R, Martin, R. L, Fox, D. J, Keith, T, Al-Laham, M. A, Peng, C. Y, Nanayakkara, A, Gonzalez, C; Challacombe, M, Gill, P. M. W, Johnson, B. G, Chen, W, Wong, M. W, Andres, J. L, Head-Gordon, M, Replogle, E. S, Pople, J. A. Gaussian 98; Gaussian, Inc, Pittsburgh, PA, 1998; Sadlej, A.J., (1995) Collect. Czech. Chem. Commun, 1988, p. 53
  • Ekstrom, C.R., Schmiedmayer, J., Chapman, M.S., Hammond, T.D., Pritchard, D.E., (1995) Phys. Rev. A, 51, p. 3883
  • Yang, M., Senet, P., Van Alsenoy, C., (2005) Int. J. Quantum Chem, 101, p. 535
  • Ghanty, T.K., Ghosh, S.K., (2003) J. Chem. Phys, 118, p. 8547
  • Rodriguez, J., Laria, D., Marceca, E., Estrin, D., (1999) J. Chem. Phys, 110, p. 9039
  • Klots, C.E., (1988) J. Phys. Chem, 92, p. 5864
  • Hashimoto, K., Morokuma, K., (1994) J. Am. Chem Soc, 116, p. 11436

Citas:

---------- APA ----------
Carrera, Á., Mobbili, M. & Marceca, E. (2009) . Electric susceptibility of sodium-doped water clusters by beam deflection. Journal of Physical Chemistry A, 113(12), 2711-2714.
http://dx.doi.org/10.1021/jp809411p
---------- CHICAGO ----------
Carrera, Á., Mobbili, M., Marceca, E. "Electric susceptibility of sodium-doped water clusters by beam deflection" . Journal of Physical Chemistry A 113, no. 12 (2009) : 2711-2714.
http://dx.doi.org/10.1021/jp809411p
---------- MLA ----------
Carrera, Á., Mobbili, M., Marceca, E. "Electric susceptibility of sodium-doped water clusters by beam deflection" . Journal of Physical Chemistry A, vol. 113, no. 12, 2009, pp. 2711-2714.
http://dx.doi.org/10.1021/jp809411p
---------- VANCOUVER ----------
Carrera, Á., Mobbili, M., Marceca, E. Electric susceptibility of sodium-doped water clusters by beam deflection. J Phys Chem A. 2009;113(12):2711-2714.
http://dx.doi.org/10.1021/jp809411p