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Soler-Illia, G.J.A.A.; Angelomé, P.C.; Fuertes, M.C.; Calvo, A.; Wolosiuk, A.; Zelcer, A.; Bellino, M.G.; Martínez, E.D. "Mesoporous hybrid and nanocomposite thin films. A sol-gel toolbox to create nanoconfined systems with localized chemical properties" (2011) Journal of Sol-Gel Science and Technology. 57(3):299-312
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Abstract:

Mesoporous Thin Films (MTF) can be created by combining sol-gel synthesis, template self-assembly and chemical surface modification. A wide palette of inorganic (oxides, phosphates, carbon-based, etc.) and hybrid organic-inorganic frameworks with a variety of composition, pore sizes, and nanoscale, organic or biological functions located in the inorganic skeleton, pore surface or pore interior can be obtained. The properties of the functional pore systems are tuned by the pore size and geometry, wall composition and surface features. These MTF with interesting electronic and optical controlled features are indeed a "nanofacility". Well-defined monodisperse sized pores also act as nanoreactors, or nanocavities with controlled environment and behaviour. In the last years, the production of accessible MTF, in which either the pore surface or pore volume can be modified by organic functional groups or nanoparticles has been thoroughly explored. Each highly controlled MTF originated from a reproducible and modular synthesis is in itself a building block for more complex structures, presenting order at different length scales (molecular, mesoscopic, macroscopic), and novel properties derived thereof. Selected examples of optical and chemical behaviour of these multiscale materials are presented to illustrate these points. © 2010 Springer Science+Business Media, LLC.

Registro:

Documento: Artículo
Título:Mesoporous hybrid and nanocomposite thin films. A sol-gel toolbox to create nanoconfined systems with localized chemical properties
Autor:Soler-Illia, G.J.A.A.; Angelomé, P.C.; Fuertes, M.C.; Calvo, A.; Wolosiuk, A.; Zelcer, A.; Bellino, M.G.; Martínez, E.D.
Filiación:Gerencia de Química, Centro Atómico Constituyentes, Comisión Nacional de Energía Atómica, Av. Gral Paz 1499 (B1650KNA), San Martín, Buenos Aires, Argentina
Departamento de Química Inorgánica, Analítica y Química Física, Facultad de Ciencias Exactas y Naturales, Ciudad Universitaria, Pabellón II, C1428EHA, Buenos Aires, Argentina
Palabras clave:Functional materials; Mesoporous films; Mesoporous hybrids; Nanochemistry; Thin films; Biological functions; Building blockes; Carbon-based; Chemical surface modification; Complex structure; Controlled environment; Different length scale; Mesoporous films; Mesoporous hybrids; Mesoporous thin films; Mesoscopics; Modular synthesis; Monodisperse; Multiscales; Nano chemistry; Nano scale; Nano-cavities; Nano-confined systems; Nanocomposite thin films; Organic functional groups; Organic-inorganic; Pore surface; Pore system; Pore volume; Selected examples; Sol-gel synthesis; Surface feature; Chemical modification; Chemical properties; Functional groups; Functional materials; Gels; Nanocomposite films; Nanocomposites; Optical transfer function; Pore size; Sol-gel process; Sol-gels; Sols; Surfaces; Thin films; Mesoporous materials
Año:2011
Volumen:57
Número:3
Página de inicio:299
Página de fin:312
DOI: http://dx.doi.org/10.1007/s10971-010-2172-2
Título revista:Journal of Sol-Gel Science and Technology
Título revista abreviado:J Sol Gel Sci Technol
ISSN:09280707
CODEN:JSGTE
Registro:https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_09280707_v57_n3_p299_SolerIllia

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Citas:

---------- APA ----------
Soler-Illia, G.J.A.A., Angelomé, P.C., Fuertes, M.C., Calvo, A., Wolosiuk, A., Zelcer, A., Bellino, M.G.,..., Martínez, E.D. (2011) . Mesoporous hybrid and nanocomposite thin films. A sol-gel toolbox to create nanoconfined systems with localized chemical properties. Journal of Sol-Gel Science and Technology, 57(3), 299-312.
http://dx.doi.org/10.1007/s10971-010-2172-2
---------- CHICAGO ----------
Soler-Illia, G.J.A.A., Angelomé, P.C., Fuertes, M.C., Calvo, A., Wolosiuk, A., Zelcer, A., et al. "Mesoporous hybrid and nanocomposite thin films. A sol-gel toolbox to create nanoconfined systems with localized chemical properties" . Journal of Sol-Gel Science and Technology 57, no. 3 (2011) : 299-312.
http://dx.doi.org/10.1007/s10971-010-2172-2
---------- MLA ----------
Soler-Illia, G.J.A.A., Angelomé, P.C., Fuertes, M.C., Calvo, A., Wolosiuk, A., Zelcer, A., et al. "Mesoporous hybrid and nanocomposite thin films. A sol-gel toolbox to create nanoconfined systems with localized chemical properties" . Journal of Sol-Gel Science and Technology, vol. 57, no. 3, 2011, pp. 299-312.
http://dx.doi.org/10.1007/s10971-010-2172-2
---------- VANCOUVER ----------
Soler-Illia, G.J.A.A., Angelomé, P.C., Fuertes, M.C., Calvo, A., Wolosiuk, A., Zelcer, A., et al. Mesoporous hybrid and nanocomposite thin films. A sol-gel toolbox to create nanoconfined systems with localized chemical properties. J Sol Gel Sci Technol. 2011;57(3):299-312.
http://dx.doi.org/10.1007/s10971-010-2172-2