Abstract:
We compute the density-fluctuation spectrum of spherical 4HeN shells adsorbed on the outer surface of C n fullerenes. The excitation spectrum is obtained within the random-phase approximation, with particle-hole elementary excitations and effective interaction extracted from a density-functional description of the shell structure. The presence of one or two solid helium layers adjacent to the adsorbing fullerene is phenomenologically accounted for. We illustrate our results for a selection of numbers of adsorbed atoms on C20, C 60, and C120. The hydrodynamical model that has proven successful to describe helium excitations in the bulk and in restricted geometries permits to perform a rather exhaustive analysis of various fluid spherical systems, namely, spheres, cavities, free bubbles, and bound shells of variable size.
Registro:
Documento: |
Artículo
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Título: | Density modes in spherical 4He shells |
Autor: | Barranco, M.; Hernández, E.S.; Mayol, R.; Pi, M. |
Filiación: | Dept. Estructura/Constituents Mat., Facultad de Física, Universitat de Barcelona, E-08028 Barcelona, Spain Departamento de Física, Fac. de Ciencias Exactas y Naturales, Universidad de Buenos Aires, 1428 Buenos Aires, Argentina Consejo Nac. de Invest. Cie. y Tec., Argentina
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Palabras clave: | carbon; fullerene; helium; article; chemical structure; density; density functional theory; elementary particle; excitation; geometry; hydrodynamics; mathematical analysis; quantum mechanics |
Año: | 2004
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Volumen: | 69
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Número: | 13
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Página de inicio: | 134502
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Página de fin: | 1-134502-10
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DOI: |
http://dx.doi.org/10.1103/PhysRevB.69.134502 |
Título revista: | Physical Review B - Condensed Matter and Materials Physics
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Título revista abreviado: | Phys. Rev. B Condens. Matter Mater. Phys.
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ISSN: | 01631829
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CODEN: | PRBMD
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CAS: | carbon, 7440-44-0; helium, 7440-59-7
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Registro: | https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_01631829_v69_n13_p134502_Barranco |
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Citas:
---------- APA ----------
Barranco, M., Hernández, E.S., Mayol, R. & Pi, M.
(2004)
. Density modes in spherical 4He shells. Physical Review B - Condensed Matter and Materials Physics, 69(13), 134502-1-134502-10.
http://dx.doi.org/10.1103/PhysRevB.69.134502---------- CHICAGO ----------
Barranco, M., Hernández, E.S., Mayol, R., Pi, M.
"Density modes in spherical 4He shells"
. Physical Review B - Condensed Matter and Materials Physics 69, no. 13
(2004) : 134502-1-134502-10.
http://dx.doi.org/10.1103/PhysRevB.69.134502---------- MLA ----------
Barranco, M., Hernández, E.S., Mayol, R., Pi, M.
"Density modes in spherical 4He shells"
. Physical Review B - Condensed Matter and Materials Physics, vol. 69, no. 13, 2004, pp. 134502-1-134502-10.
http://dx.doi.org/10.1103/PhysRevB.69.134502---------- VANCOUVER ----------
Barranco, M., Hernández, E.S., Mayol, R., Pi, M. Density modes in spherical 4He shells. Phys. Rev. B Condens. Matter Mater. Phys. 2004;69(13):134502-1-134502-10.
http://dx.doi.org/10.1103/PhysRevB.69.134502