Artículo

Ruggieri, F.; Fernandez-Turiel, J.L.; Saavedra, J.; Gimeno, D.; Polanco, E.; Amigo, A.; Galindo, G.; Caselli, A. "Contribution of volcanic ashes to the regional geochemical balance: The 2008 eruption of Chaitén volcano, Southern Chile" (2012) Science of the Total Environment. 425:75-88
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Abstract:

The environmental geochemical behaviour of the rhyolitic ashes from the 2008 eruption of Chaitén volcano, Southern Chile, has been studied. After the bulk characterisation, the potential contribution to the regional geochemical fluxes was examined using: i) single batch leaching tests to provide a rapid screening of the implied major and trace elements; and ii) column experiments to evaluate the temporal mobility of leached elements. The environmental concerns of these ashes are related to the fine grained component present in each sample (independent of distance from the source), in particular the presence of cristobalite, and the geochemical hazards posed by ash-water interaction. Leaching experiments show the fast dissolution of surface salts and aerosols, which dominate over glass dissolution during the first steps of the ash-water interaction. Chaitén ashes could transfer to the environment more than 1×10 10g or 10,000metric tonnes (mt) of Cl, S, Ca, Na, Si, and K; between 1000 and 10,000mt of F, Mg, and Al; between 100 and 1000mt of As, Pb, P, Fe, Sr, Zn, Mn, and Br; between 10 and 100mt of Ba, Li, Ti, Ni, Nb, Cu, Rb, Zr, V, Mo, Co, and Sc; and less than 10mt of Cr, Sb, Ce, Ga, Cs, and Y. These results show the fertilising potential of the ashes (e.g., providing Ca and Fe) but also the input of potentially toxic trace elements (e.g., F and As) in the regional geochemical mass balance. The Chaitén results evidence lower potentials for poisoning and fertilising than low silica ashes due to the lower contents released of practically all elements. © 2012 Elsevier B.V.

Registro:

Documento: Artículo
Título:Contribution of volcanic ashes to the regional geochemical balance: The 2008 eruption of Chaitén volcano, Southern Chile
Autor:Ruggieri, F.; Fernandez-Turiel, J.L.; Saavedra, J.; Gimeno, D.; Polanco, E.; Amigo, A.; Galindo, G.; Caselli, A.
Filiación:Institute of Earth Sciences Jaume Almera, ICTJA-CSIC, Barcelona, Spain
IRNASA-CSIC, Salamanca, Spain
Department of Geochemistry, Petrology and Geological Prospecting, Faculty of Geology, Universitat de Barcelona, Spain
Energia Andina S.A., Dario Urzua 2165, Providencia, Santiago, Chile
Servicio Nacional de Geología y Minería, SERNAGEOMIN, Casilla 10465, Santiago, Chile
Facultad de Ciencias Exactas y Naturales, Universidad de Buenos Aires, Argentina
Palabras clave:Batch leaching; Chaitén; Column leaching; Trace elements; Volcanic ash; Batch leaching; Column experiments; Column leaching; Cristobalites; Environmental concerns; Fast dissolutions; Fine-grained components; Geochemical hazard; Glass dissolution; Leaching experiments; Major and trace elements; Mass balance; Rapid screening; Rhyolitic; Toxic trace elements; Volcanic ash; Cesium; Concrete aggregates; Dissolution; Experiments; Geochemistry; Leaching; Lead; Manganese; Rubidium; Silica; Silicate minerals; Trace elements; Zirconium; Volcanoes; aluminum; antimony; barium; cerium; cesium; chromium; cobalt; gallium; iron; lithium; magnesium; manganese; molybdenum; nickel; niobium; phosphorus; potassium; rubidium; scandium; silicon; silicon dioxide; sodium; sodium chloride; strontium; titanium; vanadium; yttrium; zirconium; cristobalite; dissolution; mass balance; rhyolite; trace element; volcanic ash; volcanic eruption; volcanology; aerosol; article; biochemical composition; bioleaching; Chile; concentration (parameters); controlled study; dissolution; environmental impact assessment; environmental monitoring; geochemical analysis; geographic distribution; grain; hydrolysis; nonhuman; pH measurement; porosity; priority journal; scanning electron microscopy; social problem; surface property; volcanic ash; X ray diffraction; Chaiten Volcano; Chile; Los Lagos; Southern Volcanic Zone
Año:2012
Volumen:425
Página de inicio:75
Página de fin:88
DOI: http://dx.doi.org/10.1016/j.scitotenv.2012.03.011
Título revista:Science of the Total Environment
Título revista abreviado:Sci. Total Environ.
ISSN:00489697
CODEN:STEVA
CAS:aluminum, 7429-90-5; antimony, 14374-79-9, 7440-36-0; barium, 7440-39-3; cerium, 7440-45-1; cesium, 7440-46-2; chromium, 14092-98-9, 16065-83-1, 7440-47-3; cobalt, 7440-48-4; gallium, 14391-02-7, 7440-55-3; iron, 14093-02-8, 53858-86-9, 7439-89-6; lithium, 7439-93-2; magnesium, 7439-95-4; manganese, 16397-91-4, 7439-96-5; molybdenum, 7439-98-7; nickel, 7440-02-0; niobium, 7440-03-1; phosphorus, 7723-14-0; potassium, 7440-09-7; rubidium, 7440-17-7; scandium, 10361-84-9, 7440-20-2; silicon, 7440-21-3; silicon dioxide, 10279-57-9, 14464-46-1, 14808-60-7, 15468-32-3, 60676-86-0, 7631-86-9; sodium, 7440-23-5; sodium chloride, 7647-14-5; strontium, 7440-24-6; titanium, 7440-32-6; vanadium, 7440-62-2; yttrium, 7440-65-5; zirconium, 14940-68-2, 7440-67-7
Registro:https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_00489697_v425_n_p75_Ruggieri

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Citas:

---------- APA ----------
Ruggieri, F., Fernandez-Turiel, J.L., Saavedra, J., Gimeno, D., Polanco, E., Amigo, A., Galindo, G.,..., Caselli, A. (2012) . Contribution of volcanic ashes to the regional geochemical balance: The 2008 eruption of Chaitén volcano, Southern Chile. Science of the Total Environment, 425, 75-88.
http://dx.doi.org/10.1016/j.scitotenv.2012.03.011
---------- CHICAGO ----------
Ruggieri, F., Fernandez-Turiel, J.L., Saavedra, J., Gimeno, D., Polanco, E., Amigo, A., et al. "Contribution of volcanic ashes to the regional geochemical balance: The 2008 eruption of Chaitén volcano, Southern Chile" . Science of the Total Environment 425 (2012) : 75-88.
http://dx.doi.org/10.1016/j.scitotenv.2012.03.011
---------- MLA ----------
Ruggieri, F., Fernandez-Turiel, J.L., Saavedra, J., Gimeno, D., Polanco, E., Amigo, A., et al. "Contribution of volcanic ashes to the regional geochemical balance: The 2008 eruption of Chaitén volcano, Southern Chile" . Science of the Total Environment, vol. 425, 2012, pp. 75-88.
http://dx.doi.org/10.1016/j.scitotenv.2012.03.011
---------- VANCOUVER ----------
Ruggieri, F., Fernandez-Turiel, J.L., Saavedra, J., Gimeno, D., Polanco, E., Amigo, A., et al. Contribution of volcanic ashes to the regional geochemical balance: The 2008 eruption of Chaitén volcano, Southern Chile. Sci. Total Environ. 2012;425:75-88.
http://dx.doi.org/10.1016/j.scitotenv.2012.03.011