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Abstract:

We have developed correlations for the Henry's constant KH and the vapor-liquid distribution constant KD for 14 solutes in H2O and seven solutes in D2O. The solutes considered are common gases that might be encountered in geochemistry or the power industry. Solubility data from the literature were critically assessed and reduced to the appropriate thermodynamic quantities, making use of corrections for nonideality in the vapor and liquid phases as best they could be computed. While the correlations presented here cover the entire range of temperatures from near the freezing point of the solvent to high temperatures approaching its critical point, the main emphasis is on representation of the high-temperature behavior, making use of asymptotic relationships that constrain the temperature dependence of kH and KD near the critical point of the solvent. © 2003 by the U.S. Secretary of Commerce on behalf of the United States. All rights reserved.

Registro:

Documento: Artículo
Título:Henry's constants and vapor-liquid distribution constants for gaseous solutes in H2O and D2O at high temperatures
Autor:Fernández-Prini, R.; Alvarez, J.L.; Harvey, A.H.
Filiación:Unidad Actividad Química, Comn. Nac. de Ener. Atómica, Av. Libertador 8250, 1429 Buenos Aires, Argentina
INQUIMAE, Ftd. Ciencias Exactas y Naturales, Pabellón II, 1428 Buenos Aires, Argentina
Univ. Technológica National, Ftd. Regional Bs. As., Medrano 951, 1179 Buenos Aires, Argentina
Physical Properties Division, Natl. Inst. of Std. and Technology, 325 Broadway, Boulder, CO 80305, United States
Carrera del Investigador, CONICET, Buenos Aires, Argentina
Palabras clave:Distribution constant; Gases; Heavy water; Henry's constant; Solubility; Vapor-liquid equilibrium; Water
Año:2003
Volumen:32
Número:2
Página de inicio:903
Página de fin:916
DOI: http://dx.doi.org/10.1063/1.1564818
Título revista:Journal of Physical and Chemical Reference Data
Título revista abreviado:J. Phys. Chem. Ref. Data
ISSN:00472689
Registro:https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_00472689_v32_n2_p903_FernandezPrini

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Citas:

---------- APA ----------
Fernández-Prini, R., Alvarez, J.L. & Harvey, A.H. (2003) . Henry's constants and vapor-liquid distribution constants for gaseous solutes in H2O and D2O at high temperatures. Journal of Physical and Chemical Reference Data, 32(2), 903-916.
http://dx.doi.org/10.1063/1.1564818
---------- CHICAGO ----------
Fernández-Prini, R., Alvarez, J.L., Harvey, A.H. "Henry's constants and vapor-liquid distribution constants for gaseous solutes in H2O and D2O at high temperatures" . Journal of Physical and Chemical Reference Data 32, no. 2 (2003) : 903-916.
http://dx.doi.org/10.1063/1.1564818
---------- MLA ----------
Fernández-Prini, R., Alvarez, J.L., Harvey, A.H. "Henry's constants and vapor-liquid distribution constants for gaseous solutes in H2O and D2O at high temperatures" . Journal of Physical and Chemical Reference Data, vol. 32, no. 2, 2003, pp. 903-916.
http://dx.doi.org/10.1063/1.1564818
---------- VANCOUVER ----------
Fernández-Prini, R., Alvarez, J.L., Harvey, A.H. Henry's constants and vapor-liquid distribution constants for gaseous solutes in H2O and D2O at high temperatures. J. Phys. Chem. Ref. Data. 2003;32(2):903-916.
http://dx.doi.org/10.1063/1.1564818