Artículo
Molinero, V.; Laria, D.; Kapral, R. "Dynamics of solvation-induced structural transitions in mesoscopic binary clusters" (2000) Physical Review Letters. 84(3):455-458
Consulte la política de Acceso Abierto del editor
Abstract:
Ion solvation dynamics following collision of K+ with mesoscopic water-ammonia aggregates is investigated. Two processes determine the postcollision state of the clusters: First, a morphological transformation from a structure characterized by a solid water core and a liquid-phase ammonia sheath into a dumbbell-shaped cluster composed of a liquid water droplet attached to an ammonia subcluster containing the solvated ion. Second, evaporation cools the cluster during and after the morphological change and this evaporative cooling is quantitatively characterized by determining the size-dependent rate constants for these complex clusters. © 2000 American Physical Society.
Registro:
| Documento: | Artículo |
| Título: | Dynamics of solvation-induced structural transitions in mesoscopic binary clusters |
| Autor: | Molinero, V.; Laria, D.; Kapral, R. |
| Filiación: | Departamento de Química Inorgánica, Analítica y Química Física, Facultad de Ciencias Exactas y Naturales, Universidad de Buenos Aires, INQUIMAE, Pabellón II, Buenos Aires, 1428, Argentina Unidad Actividad Química, Comisión Nacional de Energía Atómica, Avenida del Libertador 8250, Buenos Aires, 1429, Argentina Chemical Physics Theory Group, Department of Chemistry, University of Toronto, Toronto, ONT, M5S 3H6, Canada |
| Año: | 2000 |
| Volumen: | 84 |
| Número: | 3 |
| Página de inicio: | 455 |
| Página de fin: | 458 |
| DOI: | http://dx.doi.org/10.1103/PhysRevLett.84.455 |
| Título revista: | Physical Review Letters |
| Título revista abreviado: | Phys Rev Lett |
| ISSN: | 00319007 |
| Registro: | https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_00319007_v84_n3_p455_Molinero |
Referencias:
- Sato, H., Matsuzaki, A., Nishio, S., Ito, O., Furukaewa, K., Kawasaki, T., (1998) J. Chem. Phys, 108, p. 3940
- Grégoire, G., Mons, M., Dedonder-Lardeux, C., Jouvet, C., (1998) Eur. Phys. J. D, 1, p. 5
- Choi, J.-H., Kuwata, K.T., Cao, Y.-B., Okumura, M., (1998) J. Phys. Chem, 102, p. 503
- Ayotte, P., Bailey, C.G., Weddle, G.H., Johnson, M.A., (1998) J. Phys. Chem, 102, p. 3067
- Clarke, A.S., Kapral, R., Moore, B., Patey, G., Wu, X.-G., (1993) Phys. Rev. Lett, 70, p. 3283
- Clarke, A.S., Kapral, R., Patey, G.N., (1994) J. Chem. Phys, 101, p. 2432
- Molinero, V., Laria, D., Kapral, R., (1998) J. Chem. Phys, 109, p. 6844
- Landman, U., Scharf, D., Jortner, J., (1985) Phys. Rev. Lett, 54, p. 1860
- Berendsen, H.J.C., Postma, J.P.M., Von Gunsteren, W.F., Hermans, J., (1981) Intermolecular Forces, , Reidel, Dordrecht
- Sprik, M., Impey, R., Klein, M.L., (1986) J. Am. Chem. Soc, 56, p. 2326
- Straatsma, T.P., Berendsen, H.J.C., (1988) J. Chem. Phys, 89, p. 5876
- Nosé, S., (1984) Mol. Phys, 52, p. 255
- Klots, C., (1988) J. Phys. Chem, 92, p. 5864
- Datz, S., (1982), p. 79. , North-Holland, Amsterdam; Näher, U., Hansen, K., (1994) J. Chem. Phys, 101, p. 5367
- Wei, S., Tzeng, W.B., Castleman, A.W., (1990) J. Chem. Phys, 92, p. 332
- Boon, J.P., Yip, S., (1980) Molecular Hydrodynamics, , Dover, New York, Chaps. 2 and 3
Citas:
---------- APA ----------
Molinero, V., Laria, D. & Kapral, R. (2000) . Dynamics of solvation-induced structural transitions in mesoscopic binary clusters. Physical Review Letters, 84(3), 455-458.http://dx.doi.org/10.1103/PhysRevLett.84.455
---------- CHICAGO ----------
Molinero, V., Laria, D., Kapral, R. "Dynamics of solvation-induced structural transitions in mesoscopic binary clusters" . Physical Review Letters 84, no. 3 (2000) : 455-458.http://dx.doi.org/10.1103/PhysRevLett.84.455
---------- MLA ----------
Molinero, V., Laria, D., Kapral, R. "Dynamics of solvation-induced structural transitions in mesoscopic binary clusters" . Physical Review Letters, vol. 84, no. 3, 2000, pp. 455-458.http://dx.doi.org/10.1103/PhysRevLett.84.455
---------- VANCOUVER ----------
Molinero, V., Laria, D., Kapral, R. Dynamics of solvation-induced structural transitions in mesoscopic binary clusters. Phys Rev Lett. 2000;84(3):455-458.http://dx.doi.org/10.1103/PhysRevLett.84.455
