Abstract:
The photothermal photodeflection technique is shown to provide information on the homogeneity of fuel pellets, pore distribution, clustering detection of pure urania and gadolinea and to provide a two-dimensional mapping of the thermal diffusivity correlated to the composition of the interdiffused Gadolinium and Uranium oxide. Histograms of the thermal diffusivity distribution become a reliable quantitative way of quantifying the degree of homogeneity and the width of the histogram can be used as a direct measure of the homogeneity. These quantitative measures of the homogeneity of the samples at microscopic levels provides a protocol that can be used as a reliable specification and quality control method for nuclear fuels, substituting with a single test a battery of expensive, time consuming and operator dependent techniques. © 2012 Elsevier B.V. All rights reserved.
Registro:
Documento: |
Artículo
|
Título: | Photothermal microscopy applied to the characterization of nuclear fuel pellets |
Autor: | Zaldivar Escola, F.; Martínez, O.E.; Mingolo, N.; Kempf, R. |
Filiación: | Universidad de Buenos Aires, Facultad de Ingeniería, Paseo Colon 850, 1063 Buenos Aires, Argentina Universidad de Buenos Aires, Facultad de Ciencias Exactas y Naturales Int., Cdad. Universitaria, Güiraldes 2160, Pabellón I, Caba C1428EAH, Argentina CNEA, Unidad Actividad Combustibles Nucleares, División Caracterización, San Martín, Pcia. de Buenos Aires, Argentina CONICET, Argentina Tolket SRL, Buenos Aires, Argentina
|
Palabras clave: | Direct measures; Microscopic levels; Photo-thermal; Photodeflection technique; Photothermal microscopy; Pore distribution; Quantitative measures; Two dimensional mapping; Uranium oxides; Gadolinium; Graphic methods; Statistical methods; Uranium; Nuclear fuel pellets |
Año: | 2013
|
Volumen: | 435
|
Número: | 1-3
|
Página de inicio: | 17
|
Página de fin: | 24
|
DOI: |
http://dx.doi.org/10.1016/j.jnucmat.2012.12.014 |
Título revista: | Journal of Nuclear Materials
|
Título revista abreviado: | J Nucl Mater
|
ISSN: | 00223115
|
CODEN: | JNUMA
|
Registro: | https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_00223115_v435_n1-3_p17_ZaldivarEscola |
Referencias:
- Böhm, W., Kiehlmann, H.D., Neufert, A., Peehs, M., (1987) Kerntechnik, 50, pp. 234-240
- Hellstrand, E., (1982) Trans. Am. Nucl. Soc., 40, pp. 181-185
- Skogen, F.B., Nielsen, L.A., Grummer, R.G., (1982) Trans. Am. Nucl. Soc., 40, pp. 194-198
- Assman, H., Robin, J.P., (1983) Guidebook on Quality Control of Mixed Oxides and Gadolinium Bearing Fuels for Light Water Reactors, IAEA-TECDOC-584, , IAEA Viena, Austria
- Durazzo, M., Oliveira, F.B.V., Urano De Carvalho, E.F., Riella, H.G., (2010) J. Nucl. Mater., 400, pp. 183-188
- (1995) International Atomic Energy Agency, Characteristics and Use of Urania-Gadolinia Fuels, , TECDOC-844 ISSN 1011-4289, Viena, Austria
- Hälldahl, L., Eriksson, S., (1988) J. Nucl. Mater., 153, pp. 66-70
- Martínez, O.E., Balzarotti, F., Mingolo, N., (2008) Appl. Phys. B, 90, pp. 69-77
- Crossa Archiopoli, U., Mingolo, N., Martínez, O.E., (2011) Surf. Coat. Technol., 205, pp. 3087-3092
- Crossa Archiopoli, U., Mingolo, N., Martínez, O.E., (2010) J. Appl. Phys., 107, pp. 0235201-0235206
- Bincheng, L., Roger, J.P., Pottier, L., Fournier, D., (1999) J. Appl. Phys., 86, pp. 53141-53143
- Fournier, D., (2001) MRS Bull., 26, pp. 465-470
- Rochais, D., Le Houëdec, H., Enguehard, F., Jumel, J., Lepoutre, F., (2005) J. Phys. D, 38, pp. 1498-1503
- Rosencwaig, A., Opsal, J., Smith, W.L., Willenborg, D.L., (1985) Appl. Phys. Lett., 46, pp. 1013-1015
- Rosencwaig, A., Opsal, J., Willenborg, D.L., (1983) Appl. Phys. Lett., 43, pp. 166-168
- Opsal, Rosencwaig, A., Willenborg, D.L., (1983) Appl. Opt., 22, pp. 3169-3176
- Martin, D.G., (1988) J. Nucl. Mater., 152, pp. 94-101
- Bibilashvili, Y.K., Kuleshov, A.V., Milovanov, O.V., Mikheev, E.N., Novikov, V.V., Popov, S.G., Proselkov, V.N., Godin, Yu.G., Investigation of thermal-physical and mechanical properties of uranium-gadolinium oxide fuel, IAEA-TECDOC-1416 (2003) Proceedings of A Technical Committee Meeting Brussels, pp. 85-100
- Griffiths, T.R., Hubbard, H.V.St.A., (1991) J. Nucl. Mater., 185, pp. 243-259
- Ruello, P., Becker, K.D., Ullrich, K., Desgranges, L., Petot, C., Petot-Ervas, G., (2004) J. Nucl. Mater., 328, pp. 46-54
- Singh, M.P., Thakur, C.S., Shalini, K., Banerjee, S., Bhat, N., Shivashankar, S.A., (2004) J. Appl. Phys., 96, pp. 5631-5637
- Sahoo, N.K., Thakur, S., Senthilkumar, M., Bhattacharyya, D., Das, N.C., (2003) Thin Solid Films, 440, pp. 155-168
- Ackerman, R.J., Thorn, R.J., Winslow, G.H., (1959) J. Opt. Soc. Am., 49, pp. 1107-1112
- Dakhel, A.A., (2001) J. Opt. A: Pure Appl. Opt., 3, pp. 452-454
- Fink, J.K., (2000) J. Nucl. Mater., 279, pp. 1-18
- Ronchi, C., Sheindlin, M., Musella, M., Hyland, G.J., (1999) J. Appl. Phys., 85
- Hirai, M., (1990) J. Nucl. Mater., 173, pp. 247-254
- Amaya, M., Hirai, M., Sakurai, H., Ito, K., Sasaki, M., Nomata, T., Kamimura, K., Iwasaki, R., (2002) J. Nucl. Mater., 300, pp. 57-64
Citas:
---------- APA ----------
Zaldivar Escola, F., Martínez, O.E., Mingolo, N. & Kempf, R.
(2013)
. Photothermal microscopy applied to the characterization of nuclear fuel pellets. Journal of Nuclear Materials, 435(1-3), 17-24.
http://dx.doi.org/10.1016/j.jnucmat.2012.12.014---------- CHICAGO ----------
Zaldivar Escola, F., Martínez, O.E., Mingolo, N., Kempf, R.
"Photothermal microscopy applied to the characterization of nuclear fuel pellets"
. Journal of Nuclear Materials 435, no. 1-3
(2013) : 17-24.
http://dx.doi.org/10.1016/j.jnucmat.2012.12.014---------- MLA ----------
Zaldivar Escola, F., Martínez, O.E., Mingolo, N., Kempf, R.
"Photothermal microscopy applied to the characterization of nuclear fuel pellets"
. Journal of Nuclear Materials, vol. 435, no. 1-3, 2013, pp. 17-24.
http://dx.doi.org/10.1016/j.jnucmat.2012.12.014---------- VANCOUVER ----------
Zaldivar Escola, F., Martínez, O.E., Mingolo, N., Kempf, R. Photothermal microscopy applied to the characterization of nuclear fuel pellets. J Nucl Mater. 2013;435(1-3):17-24.
http://dx.doi.org/10.1016/j.jnucmat.2012.12.014