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Ayude, M.A.; Cassanello, M.C.; Martínez, O.M.; Haure, P.M. "Phenomenological approach to interpret the effect of liquid flow modulation in trickle bed reactors at the particle scale" (2005) 7th International Conference on Gas-Liquid and Gas-Liquid-Solid Reactor Engineering. 60(22):6262-6269
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Abstract:

This work analyzes the influence of liquid flow modulation on the behavior of a reaction occurring in a spherical porous particle within a trickle bed reactor. A single first-order reaction between a gaseous reactant and a non-volatile liquid reactant is considered. Non-steady-state mass balances for gas and liquid reactants are formulated and solved under isothermal conditions in order to focus the analysis on the mass transport effects. Dynamic reactant profiles inside the catalytic particle are obtained for different cycling and system conditions. The enhancement factor (ε) due to periodic operation is defined to evaluate the impact of induced liquid flow modulation on reaction rate. Influence of cycling and system parameters on the enhancement factor is also reported for a wide range of conditions. Experimental trends observed by several authors can be explained with this approach. © 2005 Elsevier Ltd. All rights reserved.

Registro:

Documento: Artículo
Título:Phenomenological approach to interpret the effect of liquid flow modulation in trickle bed reactors at the particle scale
Autor:Ayude, M.A.; Cassanello, M.C.; Martínez, O.M.; Haure, P.M.
Filiación:INTEMA, CONICET, UNMDP, J.B. Justo 4302, 7600 Mar del Plata, Buenos Aires, Argentina
PINMATE, Dep. Industrias, FCEyN-UBA, Int. Güiraldes 2620, C1428BGA Buenos Aires, Argentina
Dep. Ing. Química, UNLP-CINDECA, Calle 47 No 257, 1900 La Plata, Argentina
Palabras clave:Chemical reactors; Liquid flow modulation; Mathematical model; Multiphase reactions; Transient response; Trickle bed reactors; Mass transportation; Porous materials; Reaction kinetics; Liquid flow modulation; Reaction rate; Trickle bed reactors; Chemical reactors; liquid flow; mathematical modeling; trickle bed reactor
Año:2005
Volumen:60
Número:22
Página de inicio:6262
Página de fin:6269
DOI: http://dx.doi.org/10.1016/j.ces.2005.03.019
Título revista:7th International Conference on Gas-Liquid and Gas-Liquid-Solid Reactor Engineering
Título revista abreviado:Chem. Eng. Sci.
ISSN:00092509
CODEN:CESCA
Registro:https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_00092509_v60_n22_p6262_Ayude

Referencias:

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Citas:

---------- APA ----------
Ayude, M.A., Cassanello, M.C., Martínez, O.M. & Haure, P.M. (2005) . Phenomenological approach to interpret the effect of liquid flow modulation in trickle bed reactors at the particle scale. 7th International Conference on Gas-Liquid and Gas-Liquid-Solid Reactor Engineering, 60(22), 6262-6269.
http://dx.doi.org/10.1016/j.ces.2005.03.019
---------- CHICAGO ----------
Ayude, M.A., Cassanello, M.C., Martínez, O.M., Haure, P.M. "Phenomenological approach to interpret the effect of liquid flow modulation in trickle bed reactors at the particle scale" . 7th International Conference on Gas-Liquid and Gas-Liquid-Solid Reactor Engineering 60, no. 22 (2005) : 6262-6269.
http://dx.doi.org/10.1016/j.ces.2005.03.019
---------- MLA ----------
Ayude, M.A., Cassanello, M.C., Martínez, O.M., Haure, P.M. "Phenomenological approach to interpret the effect of liquid flow modulation in trickle bed reactors at the particle scale" . 7th International Conference on Gas-Liquid and Gas-Liquid-Solid Reactor Engineering, vol. 60, no. 22, 2005, pp. 6262-6269.
http://dx.doi.org/10.1016/j.ces.2005.03.019
---------- VANCOUVER ----------
Ayude, M.A., Cassanello, M.C., Martínez, O.M., Haure, P.M. Phenomenological approach to interpret the effect of liquid flow modulation in trickle bed reactors at the particle scale. Chem. Eng. Sci. 2005;60(22):6262-6269.
http://dx.doi.org/10.1016/j.ces.2005.03.019